Top 6 Most Compatible Opposable Zodiac Sign Pairs for Work Libra love perfect horoscope signs are gemini, water bearer, and aries. When it comes to matters of the love, Libra seeks balance and understanding above all else. The Twins can offer excitement and playfulness to the connection, while Aquarius shares Libra's appreciation for intellect and creativity. Aries, known for their passion, can ignite a flame in Libra's being. Libra and these signs create a well-rounded and fulfilling partnership.